Using existing denominations? Restricted to Paulson THC mold:
cash:
25c -- Empress Star (blue 8V) or Four Queens (red/black half-pies)
$1 -- Jerry's Nugget (white) or Four Queens (blue quarter-pies)
$5 -- Golden Eagle or Aurora Star
$25 -- 20th Century (or Empress Star $20)
$100 -- Casablanca (showboat grey/yellow)
tourney:
25 Aviation Club de France
100 Empress Star (primary)
500 Empress Star (primary)
1000 Aurora Star
5000 Empress Star (secondary)
25000 Aviation Club de France
No more RVCL, PCA, Empress, Aztar, or Starlites in the stable, or those two mixed sets would most likely be a lot different.
However, if willing to create fantasy sets by relabeling chips.... I'd have to give that some serious thought. But I do have a relabeled 43mm IHC mold tourney set in progress that I'm pretty happy with:
T25 - Aurora Star $25
T100 - Aurora Star $100
T500 - Casino Aztar IN $1000 primary
T1000 - Aurora Star $20
T5000 - Horseshoe Cleveland $5000 secondary
T25000 - Winner's Club $10000 (47mm no-mold)
.... with the following oversize chips as backups/alternates:
Casino Aztar IN $1000 secondary (43mm)
Horseshoe Cleveland $25000 secondary (43mm)
Mandalay Bay $5 (43mm house mold)
Grand Cardroom (50mm BCC no-molds, Fire and White)